Category CH P03 Wettability Reversion in Plastics Treated with Glow Discharge

Plasmas

Abstract Corona discharge treatments are widely used to promote wettability and

adhesion in industrial processes for lamination of composite materials, as

well as application of paints, adhesives, and inks. However, the effects

of the treatment are not permanent. General industrial practice dictates

that treated plastic materials be subsequently processed within 4 hours of

treatment. In this project, I investigated the effect of corona discharge

treatment on various plastics at increasing post-treatment durations to

quantify the change in wettability over post-treatment time.

To determine how the effectiveness changes with time, I conducted

several experiments involving the measurement of contact angles of water

droplets on the surfaces of six plastic materials treated by corona

discharge plasma. These contact angles reflect the surface energies—a

measure of wettability—of the plastics, which are changed during corona

discharge treatment. Samples of widely used plastics, such as

polyethylene, polypropylene, polystyrene, polyvinylchloride, polyethylene

terephthalate, and polymethyl methacrylate, were selected. These plastic

samples were mounted on microscope slides and treated with a corona

discharge plasma for one minute. At various times after treatment, water

droplets were placed on the plastic surfaces. Image analysis of pictures

taken with a digital camera was used to determine the contact angles of

the water droplets. My study showed that the effect of increased

wettability of plastic surfaces by corona discharge treatment was not

completely irreversible. This reflects the partial reversion of the plastic

surface back to the untreated state.

The measured contact angles of all plastics slowly increased as a function

of elapsed time from two minutes to five days. This experiment showed

that, for most plastics tested, the contact angle recovered to around 50%

of the value for the untreated contact angle within 15 minutes. After four

hours, the contact angle recovered to around 65% of the value for the

untreated contact angle. After 5 days, the contact angle recovered to

around 75% of the value for the untreated contact angle. Thus,

processes which require high wettability after treatment of the materials

should take place within 15 minutes after corona discharge treatment.

However, if processes do not require such high wettability, several days

can elapse before the subsequent processes must take place. These

results have useful applications in reducing process costs and maximizing

process output in fields such the automotive, aerospace, and medical

industries.

Bibliography Ono, Shigeru, Shinriki Teii, and Shinako Takayama. Surface Treatment of

Plastic Film by Using an Atmospheric Pressure Corona Torch. HAKONE 8.

The 8th International Symposium on High Pressure Low Temperature

Plasma Chemistry. 20 Jan. 2009

<http://www.ut.ee/hakone8/papers/T7/Ono(TP).pdf>.The Plastics

Network. Corona Treatment: Why is it Necessary? The Plastics Network.

20 Jan. 2009 <http://plasticsnetwork.files.wordpress.com/2007/12/corona-

treatment.pdf>.
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